A novel integrated process for the functionalization of methane and ethane: Bromine as mediator

Lorkovic I.M., Yilmaz A., Yilmaz G.A., Zhou X.-P., Laverman L.E., Sun S., Schaefer D.J., Weiss M., Noy M.L., Cutler C.I., Sherman J.H., McFarland E.W., Stucky G.D. and Ford P.C. (2004). A novel integrated process for the functionalization of methane and ethane: Bromine as mediator. In: International Symposium on Advances in Hydroprocessing of Oil Fractions, Oaxaca Mexico, (317-322). Apr 18-22, 2004. doi:10.1016/j.cattod.2004.07.058


Author Lorkovic I.M.
Yilmaz A.
Yilmaz G.A.
Zhou X.-P.
Laverman L.E.
Sun S.
Schaefer D.J.
Weiss M.
Noy M.L.
Cutler C.I.
Sherman J.H.
McFarland E.W.
Stucky G.D.
Ford P.C.
Title of paper A novel integrated process for the functionalization of methane and ethane: Bromine as mediator
Conference name International Symposium on Advances in Hydroprocessing of Oil Fractions
Conference location Oaxaca Mexico
Conference dates Apr 18-22, 2004
Journal name Catalysis Today   Check publisher's open access policy
Publication Year 2004
Sub-type Fully published paper
DOI 10.1016/j.cattod.2004.07.058
Open Access Status Not yet assessed
ISSN 0920-5861
Volume 98
Issue 1-2 SPEC. ISS.
Start page 317
End page 322
Total pages 6
Language eng
Abstract/Summary We describe a novel, integrated multi-step process for the partial oxidation of alkanes to alcohols, ethers or olefins using O2 as oxidant. The sequential transformations are (1) alkane bromination to alkyl bromide(s) and HBr, (2) reaction of this mixture with solid metal oxide (MO) to neutralize the HBr and to generate oxygenated products or olefins plus solid metal bromide, and (3) oxidation of the spent solid with O2 to regenerate the metal oxide and Br2 for reuse.
Subjects 1503 Business and Management
1508 Process Chemistry and Technology
Keyword Alkane
Bromine-mediated
Metal oxide
Partial oxidation
Q-Index Code E1
Q-Index Status Provisional Code
Institutional Status Unknown

Document type: Conference Paper
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Created: Mon, 23 Jun 2014, 22:40:11 EST by System User