Heteroatom-Doped Graphene-Based Materials for Energy-Relevant Electrocatalytic Processes

Duan, Jingjing, Chen, Sheng, Jaroniec, Mietek and Qiao, Shi Zhang (2015) Heteroatom-Doped Graphene-Based Materials for Energy-Relevant Electrocatalytic Processes. ACS Catalysis, 5 9: 5207-5234. doi:10.1021/acscatal.5b00991

Author Duan, Jingjing
Chen, Sheng
Jaroniec, Mietek
Qiao, Shi Zhang
Title Heteroatom-Doped Graphene-Based Materials for Energy-Relevant Electrocatalytic Processes
Journal name ACS Catalysis   Check publisher's open access policy
ISSN 2155-5435
Publication date 2015-07-23
Year available 2015
Sub-type Article (original research)
DOI 10.1021/acscatal.5b00991
Open Access Status Not Open Access
Volume 5
Issue 9
Start page 5207
End page 5234
Total pages 28
Place of publication Washington, United States
Publisher American Chemical Society
Collection year 2016
Language eng
Formatted abstract
To address aggravating energy and environment issues, inexpensive, highly active, and durable electrocatalysts as noble metal substitutes both at the anode and cathode are being actively pursued. Among them, heteroatom-doped graphene-based materials show extraordinary electrocatalytic performance, some even close to or outperforming the state-of-the-art noble metals, such as Pt- and IrO2-based materials. This review provides a concise appraisal on graphene doping methods, possible doping configurations and their unique electrochemical properties, including single and double doping with N, B, S, and P. In addition, heteroatom-doped graphene-based materials are reviewed as electrocatalysts for oxygen reduction, hydrogen evolution, and oxygen evolution reactions in terms of their electrocatalytic mechanisms and performance. Significantly, three-dimensional heteroatom-doped graphene structures have been discussed, and those especially can be directly utilized as catalyst electrodes without extra binders and supports.
Keyword heteroatom-doped graphene
nonnoble electrocatalysts
oxygen reduction reaction
hydrogen evolution reaction
oxygen evolution reaction
Q-Index Code C1
Q-Index Status Provisional Code
Institutional Status Non-UQ

Document type: Journal Article
Sub-type: Article (original research)
Collections: Non HERDC
Australian Institute for Bioengineering and Nanotechnology Publications
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Citation counts: TR Web of Science Citation Count  Cited 54 times in Thomson Reuters Web of Science Article | Citations
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