Cobalt zeolites: preparation, characterization and catalytic properties for N2O decomposition

Shen, Qun, Li, Landong, He, Chi, Zhang, Xinyan, Hao, Zhengping and Xu, ZhiPing (2012) Cobalt zeolites: preparation, characterization and catalytic properties for N2O decomposition. Asia-Pacific Journal of Chemical Engineering, 7 4: 502-509.


Author Shen, Qun
Li, Landong
He, Chi
Zhang, Xinyan
Hao, Zhengping
Xu, ZhiPing
Title Cobalt zeolites: preparation, characterization and catalytic properties for N2O decomposition
Formatted title Cobalt zeolites: preparation, characterization and catalytic properties for N2O decomposition
Journal name Asia-Pacific Journal of Chemical Engineering  (ERA 2012 Listed)    (ERA 2010 Rank B)   Check publisher's open access policy
Publication date 2012-07
Sub-type Article
Year available 2012
DOI 10.1002/apj.599
Volume number 7
Issue number 4
ISSN 1932-2135; 1932-2143
Start page 502
End page 509
Total pages 8
Place of publication Chichester, West Sussex, United Kingdom
Publisher John Wiley & Sons
Collection year 2013
Language eng
Formatted abstract The current research characterized various Co/zeolite catalysts prepared by wet incipient impregnation approach and investigated their N2O catalytic decomposition activities. The Co/zeolite catalysts were characterized by BET, H2-TPR, UV–vis, NH3-TPD and TEM in detail, which reveals that the physicochemical properties of these catalysts are determined by the type of zeolite support, the cobalt species and their location (internal or external surface). In particular, it is found that the loaded cobalt species have great effects on the acidic property of zeolite supports. Co/Beta-3% shows the highest catalytic activity and the cobalt loading content slightly influences the catalytic activities of Co/Beta catalysts. Moreover, the catalytic performance of Co/Beta-3% is not disturbed by the presence of NO and O2. As thus, we believed that Beta zeolite is the most suitable support to prepare Co-loaded catalyst for N2O decomposition in our work.
Keyword Nitrous oxide
Catalytic decomposition
Cobalt oxide
zeolite
Q-Index Code C1
Q-Index Status Confirmed Code
Institutional Status UQ
Additional Notes Published online 31 May 2011

 
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